Spontaneous parametric down-conversion (also known as SPDC, parametric fluorescence or parametric scattering) is a nonlinear instant optical process that converts one photon of higher energy (namely, a ''pump'' photon) into a pair of photons (namely, ''signal'' and ''idler'' photons) of lower energy, in accordance with the laws of
energy conservation
Energy conservation is the effort to reduce wasteful energy consumption by using fewer energy services. This can be done by using energy more effectively (using less and better sources of energy for continuous service) or changing one's behavi ...
and
momentum conservation
In Newtonian mechanics, momentum (: momenta or momentums; more specifically linear momentum or translational momentum) is the Multiplication, product of the mass and velocity of an object. It is a Euclidean vector, vector quantity, possessi ...
. It is an important process in
quantum optics
Quantum optics is a branch of atomic, molecular, and optical physics and quantum chemistry that studies the behavior of photons (individual quanta of light). It includes the study of the particle-like properties of photons and their interaction ...
, for the generation of
entangled photon pairs and of single photons.
Description
A
nonlinear crystal is used to produce pairs of photons from a
photon
A photon () is an elementary particle that is a quantum of the electromagnetic field, including electromagnetic radiation such as light and radio waves, and the force carrier for the electromagnetic force. Photons are massless particles that can ...
beam. In accordance with conservations of
energy
Energy () is the physical quantity, quantitative physical property, property that is transferred to a physical body, body or to a physical system, recognizable in the performance of Work (thermodynamics), work and in the form of heat and l ...
and
momentum
In Newtonian mechanics, momentum (: momenta or momentums; more specifically linear momentum or translational momentum) is the product of the mass and velocity of an object. It is a vector quantity, possessing a magnitude and a direction. ...
, the pairs need to have combined energies and momenta equal to the energy and momentum of the original photon. Because the index of refraction changes with frequency (
dispersion), only certain triplets of frequencies will be
phase-matched so that simultaneous energy and momentum conservation can be achieved. Phase-matching is most commonly achieved using
birefringent
Birefringence, also called double refraction, is the optical property of a material having a refractive index that depends on the polarization and propagation direction of light. These optically anisotropic materials are described as birefring ...
nonlinear materials, whose index of refraction changes with polarization. As a result of this, different types of SPDC are categorized by the polarizations of the input photon (''pump'') and the two output photons (''signal'' and ''idler'').
* If the signal and idler photons share the same polarization with each other and the pump photon is destroyed, it is deemed Type-0 SPDC.
* If the signal and idler photons share the same polarization with each other, but are orthogonal to the pump polarization, it is Type-I SPDC.
* If the signal and idler photons have perpendicular polarizations, it is deemed Type II SPDC.
The conversion efficiency of SPDC is typically very low, with the highest efficiency obtained on the order of 4x10
−6 incoming photons for
PPLN in waveguides. However, if one half of the pair is detected at any time then its partner is known to be present. The degenerate portion of the output of a Type I down converter is a
squeezed vacuum that contains only even
photon
A photon () is an elementary particle that is a quantum of the electromagnetic field, including electromagnetic radiation such as light and radio waves, and the force carrier for the electromagnetic force. Photons are massless particles that can ...
number terms. The nondegenerate output of the Type II down converter is a two-mode squeezed vacuum.
Example

In a commonly used SPDC apparatus design, a strong
laser beam
A laser is a device that emits light through a process of optical amplification based on the stimulated emission of electromagnetic radiation. The word ''laser'' originated as an acronym for light amplification by stimulated emission of rad ...
, termed the "pump" beam, is directed at a BBO
(beta-barium borate) or
lithium niobate
Lithium niobate () is a synthetic salt consisting of niobium, lithium
Lithium (from , , ) is a chemical element; it has chemical symbol, symbol Li and atomic number 3. It is a soft, silvery-white alkali metal. Under standard temperatur ...
crystal. Most of the photons continue straight through the crystal. However, occasionally, some of the photons undergo spontaneous down-conversion with Type II polarization correlation, and the resultant correlated photon pairs have trajectories that are constrained along the sides of two
cone
In geometry, a cone is a three-dimensional figure that tapers smoothly from a flat base (typically a circle) to a point not contained in the base, called the '' apex'' or '' vertex''.
A cone is formed by a set of line segments, half-lines ...
s whose axes are symmetrically arranged relative to the pump beam. Due to the conservation of momentum, the two photons are always symmetrically located on the sides of the cones, relative to the pump beam. In particular, the trajectories of a small proportion of photon pairs will lie simultaneously on the two lines where the surfaces of the two cones intersect. This results in entanglement of the polarizations of the pairs of photons emerging on those two lines. The photon pairs are in an equal weight quantum superposition of the unentangled states
and
, corresponding to polarizations of left-hand side photon, right-hand side photon.
Another crystal is KDP (
potassium dihydrogen phosphate) which is mostly used in Type I down conversion, where both photons have the same polarization.
Some of the characteristics of effective parametric down-converting nonlinear crystals include:
# Nonlinearity: The
refractive index
In optics, the refractive index (or refraction index) of an optical medium is the ratio of the apparent speed of light in the air or vacuum to the speed in the medium. The refractive index determines how much the path of light is bent, or refrac ...
of the crystal changes with the intensity of the incident light. This is known as the nonlinear optical response.
# Periodicity: The crystal has a regular, repeating structure. This is known as the
lattice structure, which is responsible for the regular arrangement of the atoms in the crystal.
#
Optical anisotropy (or birefringence): The crystal has different refractive indices along different crystallographic axes.
# Temperature and pressure sensitivity: The nonlinearity of the crystal can change with temperature and pressure, and thus the crystal should be kept in a stable temperature and pressure environment.
# High nonlinear coefficient: Large nonlinear coefficient is desirable, this allow to generate a high number of entangled photons.
# High
optical damage threshold: Crystal with high optical damage threshold can endure high intensity of the pumping beam.
# Transparency in the desired wavelength range: It is important for the crystal to be transparent in the wavelength range of the pump beam for efficient nonlinear interactions
# High optical quality and low absorption: The crystal should be high optical quality and low absorption to minimize loss of the pump beam and the generated entangled photons.
History
SPDC was demonstrated as early as 1967 by
S. E. Harris, M. K. Oshman, and
R. L. Byer, as well as by D. Magde and H. Mahr. It was first applied to experiments related to
coherence by two independent pairs of researchers in the late 1980s:
Carroll Alley and Yanhua Shih, and
Rupamanjari Ghosh and
Leonard Mandel
Leonard Mandel (May 9, 1927 – February 9, 2001) was an American physicist who contributed to the development of theoretical and experimental modern optics and is widely considered one of the founding fathers of the field of quantum optics. With ...
. The
duality between incoherent (
Van Cittert–Zernike theorem) and biphoton emissions was found.
Applications
SPDC allows for the creation of
optical fields containing (to a good approximation) a single photon. As of 2005, this is the predominant mechanism for an experimenter to create single photons (also known as
Fock states). The single photons as well as the photon pairs are often used in
quantum information
Quantum information is the information of the state of a quantum system. It is the basic entity of study in quantum information theory, and can be manipulated using quantum information processing techniques. Quantum information refers to both t ...
experiments and applications like
quantum cryptography
Quantum cryptography is the science of exploiting quantum mechanical properties to perform cryptographic tasks. The best known example of quantum cryptography is quantum key distribution, which offers an information-theoretically secure soluti ...
and
Bell test experiments.
SPDC is widely used to create pairs of entangled photons with a high degree of spatial correlation.
Such pairs are used in
ghost imaging, in which information is combined from two light detectors: a conventional, multi-pixel detector that does not view the object, and a single-pixel (bucket) detector that does view the object.
Alternatives
The newly observed effect of
two-photon emission from electrically driven semiconductors has been proposed as a basis for more efficient sources of entangled photon pairs. Other than SPDC-generated photon pairs, the photons of a semiconductor-emitted pair usually are not identical but have different energies. Until recently, within the constraints of quantum uncertainty, the pair of emitted photons were assumed to be co-located: they are born from the same location. However, a new nonlocalized mechanism for the production of correlated photon pairs in SPDC has highlighted that occasionally the individual photons that constitute the pair can be emitted from spatially separated points.
See also
*
Photon upconversion
Photon upconversion (UC) is a process in which the sequential Absorption (electromagnetic radiation), absorption of two or more photons leads to the Emission spectrum, emission of light at shorter wavelength than the excitation wavelength. It is ...
References
{{DEFAULTSORT:Spontaneous Parametric Down-Conversion
Quantum optics
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