Organic Moderated Reactor Experiment
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The Organic Moderated Reactor Experiment (OMRE) was a 16 MWt experimental
organic Organic may refer to: * Organic, of or relating to an organism, a living entity * Organic, of or relating to an anatomical organ Chemistry * Organic matter, matter that has come from a once-living organism, is capable of decay or is the product ...
nuclear reactor A nuclear reactor is a device used to initiate and control a Nuclear fission, fission nuclear chain reaction. They are used for Nuclear power, commercial electricity, nuclear marine propulsion, marine propulsion, Weapons-grade plutonium, weapons ...
that operated at the
National Reactor Testing Station Idaho National Laboratory (INL) is one of the national laboratories of the United States Department of Energy and is managed by the Battelle Energy Alliance. Historically, the lab has been involved with nuclear research, although the labor ...
from 1957 to 1963 to explore the use of
hydrocarbons In organic chemistry, a hydrocarbon is an organic compound consisting entirely of hydrogen and carbon. Hydrocarbons are examples of group 14 hydrides. Hydrocarbons are generally colourless and hydrophobic; their odor is usually faint, and may b ...
as
coolant A coolant is a substance, typically liquid, that is used to reduce or regulate the temperature of a system. An ideal coolant has high thermal capacity, low viscosity, is low-cost, non-toxic, chemically inert and neither causes nor promotes corr ...
, moderator, and reflector materials in power reactor conditions. Such organic fluids are non-corrosive, do not become highly activated under irradiation, and can operate at low pressure and moderate temperature. These characteristics were considered promising towards the goal of achieving economical commercial nuclear power. The information provided by OMRE established the credibility of the
Organic nuclear reactor An organic nuclear reactor, or organic cooled reactor (OCR), is a type of nuclear reactor that uses some form of organic fluid, typically a hydrocarbon substance like polychlorinated biphenyl (PCB), for cooling and sometimes as a neutron moderat ...
concept and led to the commercial demonstration at the
Piqua Nuclear Generating Station The Piqua Nuclear Power Facility was an organic cooled and moderated nuclear reactor which operated just outside the southern city limits of Piqua, Ohio in the United States. The plant contained a 45.5-megawatt (thermal) organically cooled and m ...
. More recently, OMRE has been cited as providing key input and motivation for modern designs of such systems, aiming to help improve performance of new and advanced
nuclear power plant A nuclear power plant (NPP), also known as a nuclear power station (NPS), nuclear generating station (NGS) or atomic power station (APS) is a thermal power station in which the heat source is a nuclear reactor. As is typical of thermal power st ...
s towards the goals of
climate change mitigation Climate change mitigation (or decarbonisation) is action to limit the greenhouse gases in the atmosphere that cause climate change. Climate change mitigation actions include energy conservation, conserving energy and Fossil fuel phase-out, repl ...
.


Design

The OMRE design efforts began in July 1955. It was originally intended to operate for 1 year. The objectives of the OMRE program were to obtain the following experimental information: # Rate of radiation and thermal neutron damage to the hydrocarbon in the reactor # Effect of this damage upon the operation of the reactor # Suitable methods for ensuring satisfactory reactor operation in the presence of damaged hydrocarbon It was neither a pilot plant nor a prototype, but rather a minimum-cost experimental facility designed to investigate the feasibility of the organic concept to power reactors. It did not have an
electric power conversion In electrical engineering, power conversion is the process of converting electric energy from one form to another. A power converter is an electrical device for converting electrical energy between alternating current (AC) and direct current ( ...
system. OMRE was designed to provide operational information on the response of
diphenyl Biphenyl (also known as diphenyl, phenylbenzene, 1,1′-biphenyl, lemonene or BP) is an organic compound that forms colorless crystals. Particularly in older literature, compounds containing the functional group consisting of biphenyl less one ...
to high nuclear radiation and thermal
neutron flux The neutron flux is a scalar quantity used in nuclear physics and nuclear reactor physics. It is the total distance travelled by all free neutrons per unit time and volume. Equivalently, it can be defined as the number of neutrons travelling ...
, with flexibility to test other polyphenyls such as
terphenyl Terphenyls are a group of closely related aromatic hydrocarbons. Also known as diphenylbenzenes or triphenyls, they consist of a central benzene ring substituted with two phenyl groups. There are three substitution patterns: ''ortho''-terpheny ...
. The design criteria stated included: # Maximum fuel surface temperature between and # Bulk coolant temperature between and # Coolant velocity in fuel plates up to # Heat rejection capacity of 16 MWt # 25 fuel elements representing a total of 20.6 kg U235 # Fuel burnup of 11.2% U235 # Average
thermal A thermal column (or thermal) is a rising mass of buoyant air, a convective current in the atmosphere, that transfers heat energy vertically. Thermals are created by the uneven heating of Earth's surface from solar radiation, and are an example ...
neutron flux The neutron flux is a scalar quantity used in nuclear physics and nuclear reactor physics. It is the total distance travelled by all free neutrons per unit time and volume. Equivalently, it can be defined as the number of neutrons travelling ...
in fuel of 2 1013 n/cm2/s at # Reactor system pressure of The fuel element was a stainless steel box in which 16 active fuel plates were held in longitudinal grooves. Each fuel plate consisted of a core of
highly enriched uranium Enriched uranium is a type of uranium in which the percent composition of uranium-235 (written 235U) has been increased through the process of isotope separation. Naturally occurring uranium is composed of three major isotopes: uranium-238 (238 ...
particles uniformly dispersed in a stainless-steel matrix, clad with
304 stainless steel SAE 304 stainless steel is the most common stainless steel. It is an alloy of iron, carbon, chromium and nickel. It is an austenitic stainless steel, and is therefore not magnetic. It is less electrically and thermally conductive than carbon s ...
and rolled into a thick, wide and fuel plate. The dimensions of the rectangular reactor core were 57 centimeters by 69 centimeters by 91 centimeters. The reactor vessel was filled with diphenyl to obtain 14 feet of radiation shielding above the reactor core at . It was pressurized up to 300 psi with the inert
nitrogen Nitrogen is a chemical element; it has Symbol (chemistry), symbol N and atomic number 7. Nitrogen is a Nonmetal (chemistry), nonmetal and the lightest member of pnictogen, group 15 of the periodic table, often called the Pnictogen, pnictogens. ...
pressurized to to prevent boiling of the hydrocarbon. The nitrogen was continuously purged from the system to sweep out any hydrogen and light hydrocarbon gases, like
methane Methane ( , ) is a chemical compound with the chemical formula (one carbon atom bonded to four hydrogen atoms). It is a group-14 hydride, the simplest alkane, and the main constituent of natural gas. The abundance of methane on Earth makes ...
or
ethane Ethane ( , ) is a naturally occurring Organic compound, organic chemical compound with chemical formula . At standard temperature and pressure, ethane is a colorless, odorless gas. Like many hydrocarbons, ethane is List of purification methods ...
, produced by the decomposition of the coolant-moderator due to
pyrolysis Pyrolysis is a process involving the Bond cleavage, separation of covalent bonds in organic matter by thermal decomposition within an Chemically inert, inert environment without oxygen. Etymology The word ''pyrolysis'' is coined from the Gree ...
and
radiolysis Radiolysis is the dissociation of molecules by ionizing radiation. It is the cleavage of one or several chemical bonds resulting from exposure to high-energy flux. The radiation in this context is associated with ionizing radiation; radiolysis is ...
and discharge it out the stack. Coolant was pumped at through an air-blast heat exchanger to dump the core heat to the atmosphere. A steam system and power conversion system were not used to simplify the construction and operation of the reactor experiment. At high temperature and under irradiation, the hydrocarbons decompose and form longer chains with increasing
molecular weight A molecule is a group of two or more atoms that are held together by Force, attractive forces known as chemical bonds; depending on context, the term may or may not include ions that satisfy this criterion. In quantum physics, organic chemi ...
. This gradually degrades the heat transfer and flow characteristics of the fluid. To mitigate this, a coolant-moderator purification ran continuously to remove any hydrocarbons that had been damaged by heat or radiation. This was accomplished with a low-pressure
distillation Distillation, also classical distillation, is the process of separating the component substances of a liquid mixture of two or more chemically discrete substances; the separation process is realized by way of the selective boiling of the mixt ...
system. All systems were constructed with
carbon steel Carbon steel is a steel with carbon content from about 0.05 up to 2.1 percent by weight. The definition of carbon steel from the American Iron and Steel Institute (AISI) states: * no minimum content is specified or required for chromium, cobalt ...
, except the reactor vessel. All systems had heaters (including
induction heating Induction heating is the process of heating electrically conductive materials, namely metals or semi-conductors, by electromagnetic induction, through heat transfer passing through an inductor that creates an electromagnetic field within the coi ...
, resistance heating, and an oil-fired heater on the air-blast heat exchangers) to bring the system above the melting temperature of the coolant-moderator.


Construction

Construction of OMRE began on June 17, 1956, and completed in May 1957. The reactor containment was partially built underground and consisted of a concrete pad and corrugated steel cylinder surrounded by compacted earth for radiation shielding. Clearing, grading, roads, walks, drainage, water supply, power substation, sanitary and process waste systems, fencing, security lighting, guard station, communications system, control and processing building, and reactor foundation excavation were performed in Phase I of the construction by the Idaho Operations Office and the Atomic Energy Commission. Some delays were encountered due to appropriations delays and a steel strike. The biggest setback was unsatisfactory performance of the control-rod drive mechanism. During testing, it became apparent that the original design would not work, and a new approach was needed. Process piping was constructed of Schedule 40
carbon steel Carbon steel is a steel with carbon content from about 0.05 up to 2.1 percent by weight. The definition of carbon steel from the American Iron and Steel Institute (AISI) states: * no minimum content is specified or required for chromium, cobalt ...
. The buildings and utilities were constructed by Wadsworth & Arrington.


Operation

The OMRE first achieved criticality on September 17, 1957, and reached full power at the beginning of February, 1958. The reactor operated in two modes: without the purification system, and with the purification system. Seventeen tests were run with the first OMRE core throughout 1958 with reactor power between 0 and 12 MWt. The first three tests were system check-out tests, covering all major systems. Subsequent tests simulated the conditions expected to be encountered in the
Piqua Nuclear Generating Station The Piqua Nuclear Power Facility was an organic cooled and moderated nuclear reactor which operated just outside the southern city limits of Piqua, Ohio in the United States. The plant contained a 45.5-megawatt (thermal) organically cooled and m ...
. Test 4 demonstrated that pyrolitic decomposition rate in external piping was negligible. Tests 5-11 measured the decomposition rate and the effect of radiation damage on coolant-moderator heat-transfer characteristics. Tests 12 and 13 tested the purification system's ability to reduce the concentration of inorganic particulate matter while also reducing the high-boiler concentration from 40% to 8%. Three fuel element failures occurred during first core operation. Two occurred in experimental low-enriched assemblies with finned
aluminum Aluminium (or aluminum in North American English) is a chemical element; it has chemical symbol, symbol Al and atomic number 13. It has a density lower than that of other common metals, about one-third that of steel. Aluminium has ...
cladding due to inadequate coolant filtration, and the third was caused by improper element seating. By the end of the first year, the core had generated 958 MW-day of energy and been in operation for 5,600 hours. An extended shutdown followed to replace the core. Problems with coolant purification complicated the operation of the OMRE reactor. The polymerization of the terphenyl coolant (Santowax OM, subsequently Santowax R) lead to fouling and blockage of coolant channels and to the installation of an on-line coolant purification system. These complications and the progress of the water-cooled nuclear reactor technology led to the decision of
US Atomic Energy Commission The United States Atomic Energy Commission (AEC) was an agency of the United States government established after World War II by the U.S. Congress to foster and control the peacetime development of atomic science and technology. President Harry S. ...
to reduce the American organic nuclear reactor program on December 10, 1962, and ultimately to shutdown OMRE on June 30, 1963. The Experimental Organic Cooled Reactor (EOCR) was built next to OMRE in anticipation of further development of the concept. During the final stages of its construction, EOCR was also placed in standby and never operated.


Decommissioning

Immediately following final OMRE shutdown, the nuclear fuel and reactor vessel internals were removed, and the organic coolant Santowax R (a commercial name of a mixture of terphenyl and diphenyl isomers) was drained from all the systems and remained in this deactivated condition until 1977. The facility was eventually decontaminated and decommissioned between October 1977 and September 1979. The process was complicated by the existence of some remaining toxic and flammable Santowax-R and
xylene In organic chemistry, xylene or xylol (; IUPAC name: dimethylbenzene) are any of three organic compounds with the formula . They are derived from the substitution of two hydrogen atoms with methyl groups in a benzene ring; which hydrogens are su ...
, a neutron-activated radioactive vessel emitting 350 R/h, and
asbestos Asbestos ( ) is a group of naturally occurring, Toxicity, toxic, carcinogenic and fibrous silicate minerals. There are six types, all of which are composed of long and thin fibrous Crystal habit, crystals, each fibre (particulate with length su ...
insulation. Furthermore, due to insufficient neutron shielding being included in the design, "an extraordinary, unexpected amount of activated rock and soil was removed. The surface radiation of the excavation and backfill material was brought to 20 R/h or less, and the nuclide content of the backfill soil was brought below 0.5
pCi PCI may refer to: Business and economics * Payment card industry, businesses associated with debit, credit, and other payment cards ** Payment Card Industry Data Security Standard, a set of security requirements for credit card processors * Prov ...
/g. The decommissioning effort was initially estimated in 1977 to cost and take 2 years, and was completed on time and under budget, for a total cost of .


References


External links


Organic Moderated Reactor Experiment (1958 documentary film)

Organic cooled reactors: Five Fast Facts
(2019 American Nuclear Society article) {{Nuclear fission reactors 1958 in science Nuclear reactors Idaho National Laboratory Science experiments